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First photons and set-ups for SIRIUS beamline

SOLEIL Company Contents > All the news > News 2010 > SIRIUS - First photons and set-ups

SIRIUS beamline received its first photons in the night of 1st December, 2010. And, since November 2010, the SIRIUS experimental hutch houses the beamline diffractometer, which will allow future grazing incidence X-ray scattering experiments on surfaces (diffraction, small-angle scattering and fluorescence) at fixed energy, under resonant conditions, or in energy scanning mode. The strong point of the diffractometer is that these measurements can be performed simultaneously on the same sample using both its detector arms.

Faiceau-Imageur-SIRIUS
 
A “multi-functional” diffractometer

The first set-up allows samples weighting up to 20 kg to be positioned extremely precisely: the four-circle Kappa head positions the sample to up to 1/1000th of a degree. A baby chamber equipped with an oven mounted on the Kappa head will permit solid samples to be measured under UHV and thermal treatments to be carried out in situ.

It is equally possible to replace this Kappa head with a tower that can accept, this time, configurations up to 200 kg. This set-up allows complete freedom in sample positioning, with micron accuracy for translations and to 1/1000th degree for rotations. A Langmuir trough can be adapted to this tower for experiments on liquid surfaces and interfaces, monolayers and organic films. It is planned to mount on the tower a small reactor for the synthesis of semi-conductors and nanomaterials (MOCVD - Metal-Organic Chemical Vapor Deposition technique).

It will then be possible to analyze monocrystals, solid samples, organic layers on solids or liquids, and liquid crystals using detectors placed on the two arms of the diffractometer.

  

Complementarity between beamlines at SOLEIL

The absorption edges accessible on SIRIUS are complementary to those accessible on SAMBA, SIXS and SEXTANTS: on SIRIUS, it is the soft X-rays range that is covered (1.4 – 11 keV). This range is of interest particularly to scientists in the field of soft materials (Ca, Cl, Cd, S, P, K…), semi-conductors (K-edges of P, Si, Al, L-edges of In, Sb) and magnetism (L-edge, M-edge of 4d-5d elements, K-edge of 3d elements).

This complementarity between the lines is also reflected in the choice of equipment for SIRIUS. Indeed, besides the diffractometer which should satisfy the needs of most users of SIRIUS, the "RESOXS" reflectometer of SEXTANTS, which allows the magnetic properties of nanoparticles to be analyzed by X-ray resonant magnetic scattering (XRMS), can be installed on SIRIUS. RESOXS will therefore spend a few weeks each year in the SIRIUS experimental hutch to make higher energy measurements than on SEXTANTS.

In addition, the light source (Apple II HU 36 undulator- the first to be installed on a short section of the storage ring, and having an equally short period) and one of the two SIRIUS monochromators was selected in order to modulate the polarization of the synchrotron radiation produced: the latter can be horizontal or vertical linear, but also circular. The monochromator that maintains the circular polarization will use multilayer gratings at very shallow groove depths and variable period. This instrument is also unique for the moment, as the grating technology that underlies its operation is usually reserved for lower energies.

 

To come...

Part of the diffractometer must still be mounted and will complement the equipment and the two monochromators will then be installed in January 2011. The optics of the beamline also includes four mirrors (focusing, harmonic rejection, deflection), which are currently at the polishing stage.

Meanwhile, SIRIUS users are expected to carry out the first experiments in March 2012!

  The SIRIUS team:
from left to right, Gianluca Ciatto, Nicolas Aubert and Philippe Fontaine.

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